In 2011, the FA WSL was formed replacing the FA Women's Premier League as the top division of women's football in England.
During the 2011 season, Little was the second-leading scorer in the league with nine goals.
She scored a brace during a match against Doncaster Belles on 7 May 2011.
Arsenal finished at the top of the league table with a 10–2–2 record.
At the 2011 FA Women's Cup Final, Little was named Player of the Match and scored the opening goal in Arsenal's 2–0 win over Bristol Academy.
After the game Arsenal manager Laura Harvey described Little as "world class."

During the 2012 season, Little was the league's top scorer with 11 goals.
Arsenal clinched the regular season title with an undefeated 10–4–0 record and claimed their ninth consecutive English title.
During a match against Chelsea L.F.C. on 26 April, she scored a brace with goals in the 47th and 90th minutes helping Arsenal win 3–1.
She scored another brace during a 2–0 win against Liverpool L.F.C. on 6 May. Little was voted Women's Players' Player of the Year for 2012–13 by the Professional Footballers' Association, in the first year that the award was given to women.
Upon receiving the award, Little said, "For years, I have watched this event on television, so to come here and win the first award is fantastic."

Prior to the 2013 season, Arsenal's head coach Laura Harvey left for Seattle Reign FC in the United States.
Under new head coach Shelley Kerr, the Arsenal finished third in the regular season standings with a 10–3–1 record.
In her 14 appearances for the club, Little scored three goals.
In 2011, the FA WSL was formed replacing the FA Women's Premier League as the top division of women's football in England. During the 2011 season, Little was the second-leading scorer in the league with nine goals. She scored a brace during a match against Doncaster Belles on 7 May 2011. Arsenal finished at the top of the league table with a 10–2–2 record. At the 2011 FA Women's Cup Final, Little was named Player of the Match and scored the opening goal in Arsenal's 2–0 win over Bristol Academy. After the game Arsenal manager Laura Harvey described Little as "world class."
During the 2012 season, Little was the league's top scorer with 11 goals. Arsenal clinched the regular season title with an undefeated 10–4–0 record and claimed their ninth consecutive English title. During a match against Chelsea L.F.C. on 26 April, she scored a brace with goals in the 47th and 90th minutes helping Arsenal win 3–1. She scored another brace during a 2–0 win against Liverpool L.F.C. on 6 May. Little was voted Women's Players' Player of the Year for 2012–13 by the Professional Footballers' Association, in the first year that the award was given to women. Upon receiving the award, Little said, "For years, I have watched this event on television, so to come here and win the first award is fantastic."
Prior to the 2013 season, Arsenal's head coach Laura Harvey left for Seattle Reign FC in the United States. Under new head coach Shelley Kerr, the Arsenal finished third in the regular season standings with a 10–3–1 record. In her 14 appearances for the club, Little scored three goals.
Kim Little