Magnetic Study of the Low-Temperature Anomalies in the Optimally Doped PrBCO Compound
The anomalous magnetic properties of a nonsuperconducting PrBa<sub>2</sub>Cu<sub>3</sub>O<sub>6+</sub> <inline-formula><tex-math notation="LaTeX">$_{x}$</tex-math></inline-formula> (or PrBCO) compound in an optimally doped oxygen state of concentration (<inline-formula><tex-math notation="LaTeX">$x= {\text{0.95}}$</tex-math> </inline-formula>) are investigated at low temperatures using magnetic measurements such paraprocess magnetic susceptibility <inline-formula><tex-math notation="LaTeX">$\chi _{{\text{H}}}(T)$</tex-math></inline-formula> under different values of a DC magnetic field <italic>H</italic> up to 8 T and isothermal magnetizations <inline-formula> <tex-math notation="LaTeX">$M_{{\text{T}}}(H)$</tex-math></inline-formula> with <italic>H</italic> up to 2.1 T. The temperature dependences of the derivatives of <inline-formula><tex-math notation="LaTeX">$\chi _{{\text{H}}}(T)$ </tex-math></inline-formula> indicate a significant decrease with increasing <italic>H</italic> of the Néel temperature <inline-formula><tex-math notation="LaTeX">$T_{{\text{N}}}= {\text{14}}\,{\text{K}}$</tex-math> </inline-formula> associated with antiferromagnetic (AFM) Pr ordering. The AFM-paramagnetic phase transition remains well defined even at 8 T, whereas the small anomaly at <inline-formula><tex-math notation="LaTeX">$T_{2}= {\text{10.5}}\,{\text{K}}$</tex-math></inline-formula>, which is due to the spin reorientation phase transition already reported before, seems clearly highlighted at 2 T but entirely suppressed above 6 T. A weak ferromagnetic (WFM) contribution is revealed below <inline-formula><tex-math notation="LaTeX">$T_{{\text{N}}}$</tex-math> </inline-formula> with more evidence particularly below the low critical point <inline-formula> <tex-math notation="LaTeX">$T_{{\text{cr}}}= {\text{4-5 K}}$</tex-math></inline-formula> whose anomaly is still visible with increasing <italic>H</italic> up to 8 T. Weak field-induced transitions between AFM and WFM phases are observed in the derivatives of <inline-formula><tex-math notation="LaTeX">$M_{{\text{T}}}(H)$</tex-math></inline-formula> at a low transition field (<inline-formula><tex-math notation="LaTeX">$H_{{\text{t}}}< {\text{1}}\,{\text{T}}$</tex-math> </inline-formula>). All results are discussed and compared with those found in previous works.
Magnetic order of Pr in PrBa2Cu3O7.
The magnetic order of Pr in nonsuperconducting PrBa{sub 2}Cu{sub 3}O{sub 7} has been studied by specific-heat, susceptibility, and neutron-diffraction measurements. The basic ordering consists of a simple antiferromagnetic arrangement, with a saturated moment of 0.24{mu}{sub {ital B}} and a Neel temperature {ital T}{sub {ital N}} of {similar to}17 K, which is two orders of magnitude higher than expected from either dipolar or Rudeman-Kittel-Kasuya-Yosida interactions alone. The small moment, along with the large value of the low-temperature electronic specific-heat coefficient {gamma} of 196 mJ/mol K{sup 2}, suggests that there is substantial {ital f}-electron character at the Fermi level.
Static and dynamic properties of the high anisotropy ferrimagnets I. Experiment
Magnetization, differential magnetic susceptibility measurements and magnetic resonance study in the millimeter wave range are presented for single crystals of Tb x Y 3-x Fe5O 12 ( x