Influence of reaction channel on the isomeric cross-section ratio
Summary The influence of reaction channel on the isomeric cross-section ratio was investigated by analysing the experimental data on the reactions 52Cr(p, n)52m,gMn, 52Cr(3He, t)52m,gMn, 54Fe(d, α)52m,gMn, 54Fe(n, t)52m,gMn and 54Fe(3He, α p)52m,gMn over the incident particle energy range extending up to 35 MeV. The influence is most pronounced when the channels differ widely, for example (p, n) and (3He, t) processes, i.e. when the reaction mechanisms are different. The nuclear model calculational code EMPIRE-II described the isomeric cross-section ratio rather well in the case of a simple nucleon emission reaction, but not when complex reaction channels were involved.
Nuclear model analysis of excitation functions of α-particle induced reactions on In and Cd up to 60MeV with relevance to the production of high specific activity 117mSn.
Excitation functions were calculated for the α-particle induced reactions 115In(α,x)117mSn, 114Cd(α,n)117mSn, 116Cd(α,3n)117mSn and natCd(α,x)117mSn to analyse the production of the medically important 117mSn (T½ = 13.6 d). For calculations three nuclear model codes (i.e. TALYS, EMPIRE and ALICE-IPPE) were used and the results were compared with the available experimental data. For the most important reaction, 116Cd(α,3n)117mSn, evaluated data are presented. The yield and radionuclidic purity of 117mSn from each reaction are discussed.
Investigations of (n,t) cross sections at 14.7 MeV
Abstract The ( n, t ) reaction cross sections have been measured at E n = 14·7 MeV for 5 isotopes and 7 elements, between A = 9 and 103 using the tritium beta counting technique. The ( n, t ) reaction cross sections show a general trend to decrease with increasing atomic number. Results are compared with statistical model predictions.