Wavelength-based neutron/gamma ray discrimination in CLYC
We investigated the optical components of Cs2LiYCl6:Ce (CLYC) as a possible path to particle discrimination by measuring the effects of optical filters on the shape of the waveform and comparing filtered waveforms to unfiltered ones. Crystals packaged with two optical windows were viewed by two photomultiplier tubes operated in coincidence to be certain that the signals from the same event were analyzed. We applied long-pass optical filters with cut-off wavelengths from 280 to 455 nm, and bandpass filters with cut-off wavelengths at 313, 350, 385, and 425 nm. Waveforms from gamma rays were significantly sharpened by the 313 nm bandpass filter because this filter cut out self-trapped exciton luminescence, while neutron waveforms were largely unaffected by filtering. Cumulative distribution functions generated from average filtered waveforms indicate that the neutron/gamma assignment can be made 44 ns by applying a Kolmogorov-Smirnov test comparing an acquired waveform to the average filtered waveforms.
Analysis and comparison of the Core-to-Valence Luminescence mechanism in a large CLYC crystal under neutron and γ-ray irradiation through optical filtering selection of the scintillation light
Abstract 7Li enriched Cs2LiYCl6:Ce3+ (CLYC) is a promising inorganic scintillator for real-time γ-ray and fast neutron spectrometry. The neutron/γ-ray discrimination is usually accomplished exploiting the different quenching effects of high Linear Energy Transfer (LET) particles on different scintillation mechanisms, usually by means of the time analysis of the pulse shape. In principle, the emission wavelength information could be used to address the same task. However, a systematic study of the correlations between the CLYC decay time, its radio-luminescence spectrum and the LET of the impinging particle has not yet been performed. We therefore investigated the CLYC scintillation process under neutron and γ-ray irradiation, correlating the time response to the scintillation wavelength spectrum using a 1–inch right cylinder > 99% 7Li enriched CLYC. We found that the relative intensity of the Core to Valence Luminescence (CVL) is almost constant with photons in the energy range 20–660 keV, i.e. 0.5–5 keV/μm LET, and is only partially quenched by neutrons. Instead, the direct electron-hole capture scintillation mechanism is completely cut under neutron irradiation. The luminescence in between the deep-Ultraviolet and the Near Ultraviolet region (250-350 nm) might be attributed to both the CVL and the host luminescence, also in thick highly Ce3+-doped crystals.
Aspects of GEANT4 Monte-Carlo calculations of the BC501A neutron detector
Abstract The response function of a commercial 2 in.×2 in. BC501A neutron detector has been studied through the general-purpose Monte-Carlo (MC) simulation toolkit GEANT4. For neutron energies below 8 MeV, where the dominant detection mechanism originates from the knockout protons, the results of MC calculations reproduce remarkably well the experimental pulse-height spectra. This is not the case, however, at higher neutron energies, where the contribution of heavier charged particles to the detection mechanism becomes significant. The calculated detector efficiency is also compared at three indicative energies to the experimental one via the neutron activation technique.