Coherent crystallization of bismuth under strong excitation by ultrashort laser pulses
By means of coherent control, fully symmetric bismuth phonons A1og are investigated at helium temperature depending on the degree of crystal excitation. It is shown that coherent phonons with large amplitude show phase rigidity that is absent at small amplitude. Such a change in the phase properties of crystal lattice excitations can be understood using the concept of a coherent crystal, the achievement of which results from condensation of phonon modes arising with increasing degree of excitation.