119272921
Single-shot measurement of free-electron laser polarization at SDUV-FEL
In this paper, a division-of-amplitude photopolarimeter (DOAP) for measuring the polarization state of a free-electron laser (FEL) pulse is described. The incident FEL beam is divided into four separate beams, and four Stokes parameters can be measured in a single-shot. In the crossed-planar undulators experiment at the Shanghai deep ultraviolet FEL test facility, this DOAP instrument constructed in house responsed accurately and timely while the polarization-state of fully coherent FEL pulses were switched, which is helpful for confirming the crossed-planar undulators technique for short-wavelength FELs.
119212313
FEL Polarization Control Studies on Dalian Coherent Light Source
The polarization switch of a free-electron laser (FEL) is of great importance to the user scientific community. In this paper, we investigate the generation of controllable polarization FEL from two well-known approaches for Dalian coherent light source, i.e., crossed planar undulator and elliptical permanent undulator. In order to perform a fair comparative study, a one-dimensional time-dependent FEL code has been developed, in which the imperfection effects of an elliptical permanent undulator are taken into account. Comprehensive simulation results indicate that the residual beam energy chirp and the intrinsic FEL gain may contribute to the degradation of the polarization performance for the crossed planar undulator. And the elliptical permanent undulator is not very sensitive to the undulator errors and beam imperfections. Meanwhile, with proper configurations of the main planar undulators and additional elliptical permanent undulator section, circular polarized FEL with pulse energy exceeds 100 μJ could be achieved at Dalian coherent light source.
119256536
Polarization switching demonstration using crossed-planar undulators in a seeded free-electron laser
Polarization switching of light sources is required over a wide spectral range to investigate the symmetry of matter. In this paper, we report the first experimental demonstration of the crossed-planar undulators technique at a seeded free-electron laser, which holds great promise for the full control and fast switching of the polarization of short-wavelength radiation. In the experiment, the polarization state of the coherent radiation at the secondharmonic of the seed laser is switched successfully. The experimental results confirm the theory and pave the way for applying the crossed-planar undulators technique for seeded x-ray free-electron lasers.
119534509
Measurement of the average local energy spread of electron beam via coherent harmonic generation
The local energy spread of electron beam is a very important parameter for high-gain free-electron lasers (FELs), especially the seeded FELs. Highly accurate measurement of the extremely small local energy spread is rather challenging. In this paper, a simple method to accurately measure the average local energy spread based on the coherent harmonic generation is proposed. A one-dimensional analytical estimation is given to show the principle of this method, and three-dimensional simulation codes have been used to verify the theory. This method has been demonstrated on the Shanghai deep ultraviolet FEL, and the results show that the average local energy spread is about only 1.2 keV at the exit of the 136 MeV linac, which agrees well with the numerical simulations.
118693453
Nonintersecting Brownian motions on the unit circle. Part I: noncritical cases
117846823
Chemical Constraints on the Oxygen Abundances in Jupiter and Saturn
We perform a comparative analysis of the chemical kinetics of CO and $\rm PH_3$ in Jupiter and Saturn to assess the full set of constraints available on the troposphere water abundance in the two giant planets. For carbon monoxide we employ both a widely used CO kinetic scheme from Yung et al, and a newly identified CO chemical scheme from Visscher and Moses. For $\rm PH_3$ chemical scheme, we use the same chemical scheme as in Visscher and Fegley. Yung's chemical scheme for CO yields a water enrichment of 0.95 - 23.0 times solar abundance on Jupiter, and an upper limit of 14.0 for Saturn. Visscher's chemical scheme in contrast produces a water enrichment of 0.24 - 2.6 times solar abundance in Jupiter, and for Saturn an upper limit for water enrichment of 8.0. From this scheme, which takes advantage of the most up-to-date kinetics, we preclude high water enrichments on Jupiter and Saturn, and show that the kinetics approach yields Jovian bulk abundance in which values of C/O elevated relative to solar are admissible. Our result is consistent with recent reinterpretation of Galileo Probe data in which Jupiter formed in a water-depleted portion of the protoplanetary disk (Mousis et al).
189801755
Commissioning Results of the ReA RFQ at MSU*
The Facility for Rare Isotope Beams (FRIB) is currently in the preliminary design phase at Michigan State University (MSU). FRIB consists of a driver LINAC for the acceleration of heavy ion beams, followed by a fragmentation target station and a ReAccelerator facility (ReA3). ReA3 comprises gas stopper systems, an Electron Beam Ion Trap (EBIT) charge state booster, a room temperature radio frequency quadrupole (RFQ), a LINAC using superconducting quarter wave resonators and an achromatic beam transport and distribution line to the new experimental area. Beams from ReA3 will range from 3 MeV/u for heavy ions to about 6 MeV/u for light ions. The ReA3 RFQ, which is of the 4 rod type, is designed to accelerate ions with an Q/A of 0.2 to 0.5 from 12 keV/u to 600 keV/u. The RFQ operates at a frequency of 80.5 MHz and power levels up to 120 kW at 10% duty factor. In this paper we will report on commissioning results from the ReA3 RFQ using H2 and He beam from an auxiliary ion source.
119215029
Generating polarization controllable FELs at Dalian coherent light source
The property of the FEL polarization is of great importance to the user community. FEL pulses with ultra-high intensity and flexible polarization control ability will absolutely open up new scientific realms. In this paper, several polarizationcontrolapproachesare presentedto investigate the great potential on Dalian coherent light source, which is a government-approvednovel FEL user facility with the capability of wavelength continuously tunable in the EUV regime of 50 − 150 nm. The numerical simulations show that both circularly polarized FELs with highly modulating frequencyand 100 μJ levelpulse energycouldbe generated at Dalian coherent light source.
53997503
A PERMANENT MAGNET PHASE SHIFTER FOR THE EUROPEAN X-RAY FREE ELECTRON LASER
In undulator systems with adjustable gaps phase shifters are needed to exactly control the phase retardation between electrons and the radiation field over the entire length of an undulator system. A phase shifter based on Permanent Magnet technology for the use in the European XFEL has been developed and tested. Specifications are given. This paper will explain its magnetic principle and design. Magnetic test results are presented and thoroughly discussed. Special attention is given to the operation in the XFEL.
2277847
OPTIMIZATION AND MODELING OF THE ACCELERATOR FOR THE FERMI @ ELETTRA FEL
Design studies are in progress to use the existing FERMI{at}Elettra linear accelerator for a seeded harmonic cascade free-electron laser (FEL) facility [1]. This accelerator will be upgraded to 1.2 GeV and equipped with a low-emittance RF photocathode gun, laser heater, two bunch compressors, and a beam delivery system. We present an optimization study of all the components downstream of the gun, aimed at achieving the high peak current, low energy spread and low emittance electron beam necessary for the FEL. Various operational scenarios are discussed. Results of accelerator simulations including effects of space charge, coherent synchrotron radiation and wakefields are reported.
13174963
(TAML)FeIV O complex in aqueous solution: synthesis and spectroscopic and computational characterization.
Recently, we reported the characterization of the S = (1)/ 2 complex [Fe (V)(O)B*] (-), where B* belongs to a family of tetraamido macrocyclic ligands (TAMLs) whose iron complexes activate peroxides for environmentally useful applications. The corresponding one-electron reduced species, [Fe (IV)(O)B*] (2-) ( 2), has now been prepared in >95% yield in aqueous solution at pH > 12 by oxidation of [Fe (III)(H 2O)B*] (-) ( 1), with tert-butyl hydroperoxide. At room temperature, the monomeric species 2 is in a reversible, pH-dependent equilibrium with dimeric species [B*Fe (IV)-O-Fe (IV)B*] (2-) ( 3), with a p K a near 10. In zero field, the Mössbauer spectrum of 2 exhibits a quadrupole doublet with Delta E Q = 3.95(3) mm/s and delta = -0.19(2) mm/s, parameters consistent with a S = 1 Fe (IV) state. Studies in applied magnetic fields yielded the zero-field splitting parameter D = 24(3) cm (-1) together with the magnetic hyperfine tensor A/ g nbeta n = (-27, -27, +2) T. Fe K-edge EXAFS analysis of 2 shows a scatterer at 1.69 (2) A, a distance consistent with a Fe (IV)O bond. DFT calculations for [Fe (IV)(O)B*] (2-) reproduce the experimental data quite well. Further significant improvement was achieved by introducing hydrogen bonding of the axial oxygen with two solvent-water molecules. It is shown, using DFT, that the (57)Fe hyperfine parameters of complex 2 give evidence for strong electron donation from B* to iron.