Zeolite Apgiia for Adsorption Based Carbon Dioxide Capture
Zhen Liu, Chunzhi Shen, Filipe V.S. Lopes, Ping Li, Jianguo Yu, Carlos A. Grande, Alirio E. Rodrigues
Adsorption of synthetic flue gas on a commercial zeolite 13X (APGIIA) with targeted Si/Al ratio has been studied aiming to design an adsorption process for CO2 capture from post-combustion power plants. Adsorption equilibrium of pure gases (CO2 and N2) has been measured in a wide range of temperatures: 303, 333, 363, 393, 423, 473 K. Adsorption equilibrium was fitted with the multisite Langmuir model. The adsorption capacity of the zeolite pellets for CO2 is 4.54 mol/kg and 0.26 mol/kg for N2 at 303 K and 100 kPa. The dynamic behavior of the pellets in a fixed bed was also studied by measuring breakthrough curves. Adsorption and desorption was analyzed in order to understand the regeneration of the adsorbent.Based on equilibrium and kinetic data, two different adsorption technologies were simulated: Vacuum Pressure Swing Adsorption (VPSA) and Temperature Swing Adsorption (TSA). A CO2 recovery of 63.0% with 72.1% purity was obtained using a five-step PSA cycle included rinse step. In a 5-step TSA process, however, a CO2 purity of 78.7% and recovery of 76.6% can be achieved under a heating temperature of 423 K. © 2013 Copyright Taylor and Francis Group, LLC.
Separation Science and Technology (Philadelphia)
Generated from Scopus record by KAUST IRTS on 2022-09-13
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Carbon Dioxide Chemistry 100%
Adsorption Material Science 100%
Zeolite Chemistry 37%
Reaction Temperature Chemistry 37%
Purity Chemistry 37%
Equilibrium Chemistry 37%
Temperature Engineering 37%
Mols Engineering 25%
Liu, Z., Shen, C., Lopes, F. V. S., Li, P., Yu, J., Grande, C. A., & Rodrigues, A. E. (2013). Zeolite Apgiia for Adsorption Based Carbon Dioxide Capture. Separation Science and Technology (Philadelphia), 48(3), 388-402. https://doi.org/10.1080/01496395.2012.703751
Liu, Zhen ; Shen, Chunzhi ; Lopes, Filipe V.S. et al. / Zeolite Apgiia for Adsorption Based Carbon Dioxide Capture. In: Separation Science and Technology (Philadelphia). 2013 ; Vol. 48, No. 3. pp. 388-402.
@article{072439b606324e4c8b8b18be9673e4ef,
title = "Zeolite Apgiia for Adsorption Based Carbon Dioxide Capture",
abstract = "Adsorption of synthetic flue gas on a commercial zeolite 13X (APGIIA) with targeted Si/Al ratio has been studied aiming to design an adsorption process for CO2 capture from post-combustion power plants. Adsorption equilibrium of pure gases (CO2 and N2) has been measured in a wide range of temperatures: 303, 333, 363, 393, 423, 473 K. Adsorption equilibrium was fitted with the multisite Langmuir model. The adsorption capacity of the zeolite pellets for CO2 is 4.54 mol/kg and 0.26 mol/kg for N2 at 303 K and 100 kPa. The dynamic behavior of the pellets in a fixed bed was also studied by measuring breakthrough curves. Adsorption and desorption was analyzed in order to understand the regeneration of the adsorbent.Based on equilibrium and kinetic data, two different adsorption technologies were simulated: Vacuum Pressure Swing Adsorption (VPSA) and Temperature Swing Adsorption (TSA). A CO2 recovery of 63.0% with 72.1% purity was obtained using a five-step PSA cycle included rinse step. In a 5-step TSA process, however, a CO2 purity of 78.7% and recovery of 76.6% can be achieved under a heating temperature of 423 K. {\textcopyright} 2013 Copyright Taylor and Francis Group, LLC.",
author = "Zhen Liu and Chunzhi Shen and Lopes, {Filipe V.S.} and Ping Li and Jianguo Yu and Grande, {Carlos A.} and Rodrigues, {Alirio E.}",
note = "Generated from Scopus record by KAUST IRTS on 2022-09-13",
journal = "Separation Science and Technology (Philadelphia)",
Liu, Z, Shen, C, Lopes, FVS, Li, P, Yu, J, Grande, CA & Rodrigues, AE 2013, 'Zeolite Apgiia for Adsorption Based Carbon Dioxide Capture', Separation Science and Technology (Philadelphia), vol. 48, no. 3, pp. 388-402. https://doi.org/10.1080/01496395.2012.703751
Zeolite Apgiia for Adsorption Based Carbon Dioxide Capture. / Liu, Zhen; Shen, Chunzhi; Lopes, Filipe V.S. et al.
In: Separation Science and Technology (Philadelphia), Vol. 48, No. 3, 01.01.2013, p. 388-402.
T1 - Zeolite Apgiia for Adsorption Based Carbon Dioxide Capture
AU - Liu, Zhen
AU - Shen, Chunzhi
AU - Lopes, Filipe V.S.
AU - Li, Ping
AU - Yu, Jianguo
AU - Grande, Carlos A.
AU - Rodrigues, Alirio E.
N1 - Generated from Scopus record by KAUST IRTS on 2022-09-13
N2 - Adsorption of synthetic flue gas on a commercial zeolite 13X (APGIIA) with targeted Si/Al ratio has been studied aiming to design an adsorption process for CO2 capture from post-combustion power plants. Adsorption equilibrium of pure gases (CO2 and N2) has been measured in a wide range of temperatures: 303, 333, 363, 393, 423, 473 K. Adsorption equilibrium was fitted with the multisite Langmuir model. The adsorption capacity of the zeolite pellets for CO2 is 4.54 mol/kg and 0.26 mol/kg for N2 at 303 K and 100 kPa. The dynamic behavior of the pellets in a fixed bed was also studied by measuring breakthrough curves. Adsorption and desorption was analyzed in order to understand the regeneration of the adsorbent.Based on equilibrium and kinetic data, two different adsorption technologies were simulated: Vacuum Pressure Swing Adsorption (VPSA) and Temperature Swing Adsorption (TSA). A CO2 recovery of 63.0% with 72.1% purity was obtained using a five-step PSA cycle included rinse step. In a 5-step TSA process, however, a CO2 purity of 78.7% and recovery of 76.6% can be achieved under a heating temperature of 423 K. © 2013 Copyright Taylor and Francis Group, LLC.
AB - Adsorption of synthetic flue gas on a commercial zeolite 13X (APGIIA) with targeted Si/Al ratio has been studied aiming to design an adsorption process for CO2 capture from post-combustion power plants. Adsorption equilibrium of pure gases (CO2 and N2) has been measured in a wide range of temperatures: 303, 333, 363, 393, 423, 473 K. Adsorption equilibrium was fitted with the multisite Langmuir model. The adsorption capacity of the zeolite pellets for CO2 is 4.54 mol/kg and 0.26 mol/kg for N2 at 303 K and 100 kPa. The dynamic behavior of the pellets in a fixed bed was also studied by measuring breakthrough curves. Adsorption and desorption was analyzed in order to understand the regeneration of the adsorbent.Based on equilibrium and kinetic data, two different adsorption technologies were simulated: Vacuum Pressure Swing Adsorption (VPSA) and Temperature Swing Adsorption (TSA). A CO2 recovery of 63.0% with 72.1% purity was obtained using a five-step PSA cycle included rinse step. In a 5-step TSA process, however, a CO2 purity of 78.7% and recovery of 76.6% can be achieved under a heating temperature of 423 K. © 2013 Copyright Taylor and Francis Group, LLC.
UR - http://www.tandfonline.com/doi/abs/10.1080/01496395.2012.703751
JO - Separation Science and Technology (Philadelphia)
JF - Separation Science and Technology (Philadelphia)
Liu Z, Shen C, Lopes FVS, Li P, Yu J, Grande CA et al. Zeolite Apgiia for Adsorption Based Carbon Dioxide Capture. Separation Science and Technology (Philadelphia). 2013 Jan 1;48(3):388-402. doi: 10.1080/01496395.2012.703751