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Herbs to Help Calm an Overactive Dog. Herbs are packed with vitamins, minerals, protein, carbohydrates and fat; they play a key role in your dog's overall well-being and nutrition. Herbs known for their calming properties include valerian, lemon balm, Roman chamomile, lavender, oat and skullcap.
Method 2 of 2: Calming Your Dog without Medication. 1. Make sure your dog gets plenty of exercise. Many experts on dog behavior recommend that a dog be exercised before travelling, or before being engaged in any activity that might get the dog restless and agitated.