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Herbs to Help Calm an Overactive Dog. Herbs are packed with vitamins, minerals, protein, carbohydrates and fat; they play a key role in your dog's overall well-being and nutrition. Herbs known for their calming properties include valerian, lemon balm, Roman chamomile, lavender, oat and skullcap.
Three Methods:Calming a Dog with Herbal TreatmentsProviding a Calm Environment for Your DogInteracting with Your Dog to Calm ItCommunity Q&A. When your dog is nervous or anxious, you can calm it down naturally, without the use of any medications or other artificial means.