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Herbs to Help Calm an Overactive Dog. Herbs are packed with vitamins, minerals, protein, carbohydrates and fat; they play a key role in your dog's overall well-being and nutrition. Herbs known for their calming properties include valerian, lemon balm, Roman chamomile, lavender, oat and skullcap.
Step 3. Give your dog natural herbs. Herbal supplements offer the relaxing and calming effects of natural remedies in a convenient pill form. Herbs such as valerian, St. John's wort and avena offer calming effects, and you can give them directly to your dog or mix them in his food.